Make no assumptions.
1-verify driveshafts are good, balanced perfectly, and in viable condition since they are now spinning faster.
2- verify that rear pinion angle can be dialed in by pulling the front driveshaft and doing the work and test drives.
3- Only after the rear is done should you install front and see what happens. Do the work with a mindful eye on steering and drivability. It does little good to dial out the vibes with a low caster angle and put up with shit steering.
Diagnose, hypothesize, test, use the results to create a forward path to resolution.
Can you expand on #2? Do you have a specific technique or order of operations you go through here? A commonly-successful starting point, specific range of pinion angles and increments of adjustment you go through to find the sweet spot?
-I've tried ~1° above (due to measurement error on my part thinking I was dead-even), and 0.2, 0.9, and 1.4 degrees below shaft angle with the front shaft out. It's still there, and it still pulses/oscillates.
-0.9 was the best at 71mph, but still not completely gone, and at 75mph the peak intensity doesn't seem to change with pinion angle.
-Both shafts are X splines from Tom Wood's and should be balanced as well as they can get them because I specifically asked due to running 4k+ RPM at 75mph (and because the rear was already buzzing). Rear was sent back and re-balanced again and has new straps.
-4.88 with 32's puts my driveshaft vs vehicle speed in the same neighborhood (a hair slower even) as 35/5.13, which is common in the 42RLE crowd so even though it's a weird (and temporary) combination for a NSG370, it's not outside the realm of common configurations for modified rigs.
-LJ with a JB SS SYE and stock belly skid, so my shaft is 29" long and only requires ~11° of pinion angle to be dead straight with the shaft - nowhere near the CV operating angle as the guys running full tucks on a TJ wheelbase.
-vibration is completely independent of load - on the gas, off the gas, clutch in, doesn't change.
These are the same axles (open CAD-eliminated HP 30, E-locker 44, stock shafts), transfer case, and mostly the same suspension (shortarm Savvy UCAs and JJ-retrofitted RC LCAs, Currie front and JKS rear track bars - I now have 4" currie in the front and 3" Zone plus 3/4" spacers in the rear, the TJ had unidentified 3" springs with spacers but about the same ride height), and wheels/tires that were on my '99 AX15 4.56 TJ with zero vibes. I regeared to 4.88 shortly before swapping everything over to the LJ (after my gears ate themselves and I decided to gear for 35s) but I honestly can't even remember if I got it past 60mph before tearing it down so I don't know if it started with the regear, rig swap, or driveshaft.
I know it should get better (or at least move up in vehicle speed) once I get 35's but it's still starting at low enough speeds that the 35's won't move it completely out of range.