Ok glad to find out it's the automatic as my TJ has. There is no way 4.56 will work for 33's with your 4-speed automatic like it would for a 5-speed manual transmission. In fact 4.56 is ideal for the 5-speed manual transmission and 33" tires... but not for your 4-speed automatic.
But for your 4-speed 42RLE automatic, you absolutely need 4.88 gears at a minimum but if it were me I'd go with 5.13 which is available from Revolution Gear for both your front Dana 30 and rear Dana 44. The reason your automatic needs a lower ratio (like 4.88 or 5.13) is due to its extremely steep .69 Overdrive ratio which drops the highway RPMs way too low for 4.56 to do anything but lug your engine.
I'm running 5.38 for my 35" tires and it is barely adequate but it sure works great compared to my previous 4.88 which was just terrible with 35's and my automatic.
No, 5.13 will not (!!!) make your highway RPMs too high, they'll be right in the sweet spot. In fact, when I regeared from 4.88 to 5.38 for my 35's to slightly increase the engine RPMs so the engine was no longer lugging, my MPG improved from just under 12 to just over 14 MPG. For your 33's, I definitely go with either 4.88 or 5.13 and 5.13 would be the better choice between the two... and that recommendation is based on what works best on the highway, not offroad where either would be fine.